Abstract

The nature of the pseudogap state is widely believed as a key to understanding the pairing mechanism underlying unconventional superconductivity. Over the past two decades, significant efforts have been devoted to searching for spontaneous symmetry breaking or potential order parameters associated with these pseudogap states, aiming to better characterize their properties. Recently, pseudogap states have also been realized in moiré systems with extensive gate-tunability, yet their local electronic structure remains largely unexplored. In this study, we report the observation of gate-tunable spontaneous symmetry breaking and sliding behavior of the pseudogap state in magic-angle twisted bilayer graphene (MAtBG) using spectroscopic imaging scanning tunneling microscopy. Our spectroscopy reveals a distinct pseudogap at 4.4 K within the doping range -3 < ν < -2. Spectroscopic imaging highlights a gap size modulation at moiré scale that is sensitive to the filling, indicative of a wave-like fluctuating pseudogap feature. Specifically, the positions of gap size minima (GSM) coincide with regions of the highest local density of states (LDOS) at the filling ν = -2.63, but a unidirectional sliding behavior of GSM is observed for other fillings. In addition, the pseudogap size distribution at certain doping levels also causes a clear nematic order, or an anisotropic gap distribution. Our results have shed light on the complex nature of this pseudogap state, revealing critical insights into the phase diagram of correlated electron systems.

Abstract

The nature of the pseudogap state is widely believed as a key to understanding the pairing mechanism underlying unconventional superconductivity. Over the past two decades, significant efforts have been devoted to searching for spontaneous symmetry breaking or potential order parameters associated with these pseudogap states, aiming to better characterize their properties. Recently, pseudogap states have also been realized in moiré systems with extensive gate-tunability, yet their local electronic structure remains largely unexplored. In this study, we report the observation of gate-tunable spontaneous symmetry breaking and sliding behavior of the pseudogap state in magic-angle twisted bilayer graphene (MAtBG) using spectroscopic imaging scanning tunneling microscopy. Our spectroscopy reveals a distinct pseudogap at 4.4 K within the doping range -3 < ν < -2. Spectroscopic imaging highlights a gap size modulation at moiré scale that is sensitive to the filling, indicative of a wave-like fluctuating pseudogap feature. Specifically, the positions of gap size minima (GSM) coincide with regions of the highest local density of states (LDOS) at the filling ν = -2.63, but a unidirectional sliding behavior of GSM is observed for other fillings. In addition, the pseudogap size distribution at certain doping levels also causes a clear nematic order, or an anisotropic gap distribution. Our results have shed light on the complex nature of this pseudogap state, revealing critical insights into the phase diagram of correlated electron systems.

Abstract

The nature of the pseudogap state is widely believed as a key to understanding the pairing mechanism underlying unconventional superconductivity. Over the past two decades, significant efforts have been devoted to searching for spontaneous symmetry breaking or potential order parameters associated with these pseudogap states, aiming to better characterize their properties. Recently, pseudogap states have also been realized in moiré systems with extensive gate-tunability, yet their local electronic structure remains largely unexplored. In this study, we report the observation of gate-tunable spontaneous symmetry breaking and sliding behavior of the pseudogap state in magic-angle twisted bilayer graphene (MAtBG) using spectroscopic imaging scanning tunneling microscopy. Our spectroscopy reveals a distinct pseudogap at 4.4 K within the doping range -3 < ν < -2. Spectroscopic imaging highlights a gap size modulation at moiré scale that is sensitive to the filling, indicative of a wave-like fluctuating pseudogap feature. Specifically, the positions of gap size minima (GSM) coincide with regions of the highest local density of states (LDOS) at the filling ν = -2.63, but a unidirectional sliding behavior of GSM is observed for other fillings. In addition, the pseudogap size distribution at certain doping levels also causes a clear nematic order, or an anisotropic gap distribution. Our results have shed light on the complex nature of this pseudogap state, revealing critical insights into the phase diagram of correlated electron systems.

Abstract

The nature of the pseudogap state is widely believed as a key to understanding the pairing mechanism underlying unconventional superconductivity. Over the past two decades, significant efforts have been devoted to searching for spontaneous symmetry breaking or potential order parameters associated with these pseudogap states, aiming to better characterize their properties. Recently, pseudogap states have also been realized in moiré systems with extensive gate-tunability, yet their local electronic structure remains largely unexplored. In this study, we report the observation of gate-tunable spontaneous symmetry breaking and sliding behavior of the pseudogap state in magic-angle twisted bilayer graphene (MAtBG) using spectroscopic imaging scanning tunneling microscopy. Our spectroscopy reveals a distinct pseudogap at 4.4 K within the doping range -3 < ν < -2. Spectroscopic imaging highlights a gap size modulation at moiré scale that is sensitive to the filling, indicative of a wave-like fluctuating pseudogap feature. Specifically, the positions of gap size minima (GSM) coincide with regions of the highest local density of states (LDOS) at the filling ν = -2.63, but a unidirectional sliding behavior of GSM is observed for other fillings. In addition, the pseudogap size distribution at certain doping levels also causes a clear nematic order, or an anisotropic gap distribution. Our results have shed light on the complex nature of this pseudogap state, revealing critical insights into the phase diagram of correlated electron systems.