Research paperComputational DFTComputational MDTheoreticalUpper limit of spin relaxation in suspended grapheneAron W. Cummings, Simon M.-M. Dubois, Pedro Alcázar Guerrero, Jean-Christophe Charlier et al.2024·10.13039/501100011033·arXiv:2412.11000AbstractWe use a combination of molecular dynamics and quantum transport simulations to investigate the upper limit of spin transport in suspended graphene. We find that thermally-induced atomic-scale corrugations are the dominant factor, limiting spin lifetimes to ~10 ns by inducing a strongly-varying local spin-orbit coupling. These extremely short-range corrugations appear even when the height profile appears to be smooth, suggesting they may be present in any graphene device. We discuss our results in the context of experiments, and briefly consider approaches to suppress these short-range corrugations and further enhance spin lifetimes in graphene-based spin devices.Read more
Corrugated graphene fitting structure with 1x1 unit cell used in first-principles fitting.13 propertiesSimulated Supercell DftCStudied MaterialExpand
Corrugated graphene fitting structure with 2x2 unit cell used in first-principles fitting.13 propertiesSimulated Supercell DftCStudied MaterialExpand
Thermally corrugated graphene ensemble generated at 100 K for transport averaging.1 propertySimulatedCStudied MaterialExpand
Thermally corrugated graphene ensemble generated at 200 K for transport averaging.1 propertySimulatedCStudied MaterialExpand
Thermally corrugated graphene ensemble generated at 300 K for transport averaging.1 propertySimulatedCStudied MaterialExpand
Thermally corrugated graphene ensemble generated at 400 K for transport averaging.1 propertySimulatedCStudied MaterialExpand
Research paperComputational DFTComputational MDTheoreticalUpper limit of spin relaxation in suspended grapheneAron W. Cummings, Simon M.-M. Dubois, Pedro Alcázar Guerrero, Jean-Christophe Charlier et al.2024·10.13039/501100011033·arXiv:2412.11000AbstractWe use a combination of molecular dynamics and quantum transport simulations to investigate the upper limit of spin transport in suspended graphene. We find that thermally-induced atomic-scale corrugations are the dominant factor, limiting spin lifetimes to ~10 ns by inducing a strongly-varying local spin-orbit coupling. These extremely short-range corrugations appear even when the height profile appears to be smooth, suggesting they may be present in any graphene device. We discuss our results in the context of experiments, and briefly consider approaches to suppress these short-range corrugations and further enhance spin lifetimes in graphene-based spin devices.Read more
Corrugated graphene fitting structure with 1x1 unit cell used in first-principles fitting.13 propertiesSimulated Supercell DftCStudied MaterialExpand
Corrugated graphene fitting structure with 2x2 unit cell used in first-principles fitting.13 propertiesSimulated Supercell DftCStudied MaterialExpand
Thermally corrugated graphene ensemble generated at 100 K for transport averaging.1 propertySimulatedCStudied MaterialExpand
Thermally corrugated graphene ensemble generated at 200 K for transport averaging.1 propertySimulatedCStudied MaterialExpand
Thermally corrugated graphene ensemble generated at 300 K for transport averaging.1 propertySimulatedCStudied MaterialExpand
Thermally corrugated graphene ensemble generated at 400 K for transport averaging.1 propertySimulatedCStudied MaterialExpand
Research paperComputational DFTComputational MDTheoreticalUpper limit of spin relaxation in suspended grapheneAron W. Cummings, Simon M.-M. Dubois, Pedro Alcázar Guerrero, Jean-Christophe Charlier et al.2024·10.13039/501100011033·arXiv:2412.11000AbstractWe use a combination of molecular dynamics and quantum transport simulations to investigate the upper limit of spin transport in suspended graphene. We find that thermally-induced atomic-scale corrugations are the dominant factor, limiting spin lifetimes to ~10 ns by inducing a strongly-varying local spin-orbit coupling. These extremely short-range corrugations appear even when the height profile appears to be smooth, suggesting they may be present in any graphene device. We discuss our results in the context of experiments, and briefly consider approaches to suppress these short-range corrugations and further enhance spin lifetimes in graphene-based spin devices.Read more
Corrugated graphene fitting structure with 1x1 unit cell used in first-principles fitting.13 propertiesSimulated Supercell DftCStudied MaterialExpand
Corrugated graphene fitting structure with 2x2 unit cell used in first-principles fitting.13 propertiesSimulated Supercell DftCStudied MaterialExpand
Thermally corrugated graphene ensemble generated at 100 K for transport averaging.1 propertySimulatedCStudied MaterialExpand
Thermally corrugated graphene ensemble generated at 200 K for transport averaging.1 propertySimulatedCStudied MaterialExpand
Thermally corrugated graphene ensemble generated at 300 K for transport averaging.1 propertySimulatedCStudied MaterialExpand
Thermally corrugated graphene ensemble generated at 400 K for transport averaging.1 propertySimulatedCStudied MaterialExpand
Research paperComputational DFTComputational MDTheoreticalUpper limit of spin relaxation in suspended grapheneAron W. Cummings, Simon M.-M. Dubois, Pedro Alcázar Guerrero, Jean-Christophe Charlier et al.2024·10.13039/501100011033·arXiv:2412.11000AbstractWe use a combination of molecular dynamics and quantum transport simulations to investigate the upper limit of spin transport in suspended graphene. We find that thermally-induced atomic-scale corrugations are the dominant factor, limiting spin lifetimes to ~10 ns by inducing a strongly-varying local spin-orbit coupling. These extremely short-range corrugations appear even when the height profile appears to be smooth, suggesting they may be present in any graphene device. We discuss our results in the context of experiments, and briefly consider approaches to suppress these short-range corrugations and further enhance spin lifetimes in graphene-based spin devices.Read more
Corrugated graphene fitting structure with 1x1 unit cell used in first-principles fitting.13 propertiesSimulated Supercell DftCStudied MaterialExpand
Corrugated graphene fitting structure with 2x2 unit cell used in first-principles fitting.13 propertiesSimulated Supercell DftCStudied MaterialExpand
Thermally corrugated graphene ensemble generated at 100 K for transport averaging.1 propertySimulatedCStudied MaterialExpand
Thermally corrugated graphene ensemble generated at 200 K for transport averaging.1 propertySimulatedCStudied MaterialExpand
Thermally corrugated graphene ensemble generated at 300 K for transport averaging.1 propertySimulatedCStudied MaterialExpand
Thermally corrugated graphene ensemble generated at 400 K for transport averaging.1 propertySimulatedCStudied MaterialExpand